The last piece resolving the low-mass nuclei puzzle

Using the high-precision Penning trap for light ions (LIONTRAP), physicists from MPIK and the GSI Helmholtzzentrum für Schwerionenforschung Darmstadt determined the 3He atomic mass with 12 ppt accuracy providing the last missing link between the masses in the regime of light ions. (Physical Review A, 9 April 2025; Editor’s Suggestion)

  • The mass of 3He ions is measured with 12 ppt precision directly relative to the carbon mass standard using a high-precision Penning trap.
  • The 3He atomic mass is determined to be 3.016 029 322 011(35) u.
  • The result resolves discrepancies in the reported masses of light atomic nuclei from various experiments (“low mass nuclei puzzle”).

Previous studies using the high-precision Penning trap for light ions (LIONTRAP) succeeded in measuring the masses of the proton, the deuteron and the alpha particle with unprecedented precision. However, the results differ significantly from those by the University of Washington (UW), which either contributed to or served as previous literature values while, on the other hand, agree with mass ratios measured at the Florida State University (FSU). These inconsistencies, called the “light ion mass puzzle”, are illustrated in Fig. 1.

The last missing link, a remeasurement of the 3He mass directly relative to the carbon mass standard using LIONTRAP was now performed by physicists from the Max-Planck-Institut für Kernphysik in Heidelberg (MPIK) and the GSI Helmholtzzentrum für Schwerionenforschung Darmstadt. From the the cyclotron frequency ratio of 3He+ and 12C4+ ions measured with 12 parts per trillion relative precision the atomic mass of 3He was determined to be 3.016 029 322 011(35) u.

Fig. 2 illustrates the progress in resolving the puzzle of light nuclear masses by examining the difference Δ between the summed proton (p) and deuteron (d) masses and the mass of the 3He nucleus (he). While the data solely based on the UW measurements deviate significantly the FSU values the new results from LIONTRAP and FSU are mutually consistent. Although not directly part of the puzzle, the deviation of the LIONTRAP result for the α particle (4He) reported in 2023 from the UW value supports this interpretation. Further mass measurements of light ions are planned at the PENTATRAP experiment at MPIK.


Original publication:

Penning-trap mass measurement of 3He
O. Bezrodnova, S. Sasidharan, W. Quint, S. Sturm and K. Blaum
Physical Review A 111, L040801 (2025). DOI: 10.1103/PhysRevA.111.L040801


Weblinks:

Precision mass spectrometry at MPIK


Contact

Olesia Bezrodnova
Phone: +49 6131 392-8372

Prof. Dr. Wolfgang Quint
GSI Helmholtzzentrum für Schwerionenforschung GmbH
Phone: +49 6159 71-2141

Apl. Prof. Dr.Sven Sturm
Phone: +49 6221 516-447


Press & Public Outreach

Dr. Renate Hubele / PD Dr. Bernold Feuerstein
Phone: +49 6221 516-651 / +49 6221 516-281



Figure 1: The “Light ion mass puzzle”. High-precision mass measurements by the University of Washington (UW), Florida State University (FSU) and MPIK. The conflicting results are marked by red flashes. Credit: MPIK.

Figure 2: The value of Δ = m(p) + m(d) – m(he), obtained by the University of Washington (UW), Florida State University (FSU) and MPIK (LIONTRAP). Points with error bars represent the measurements with 12C as a reference ion. The diagram on the right side indicates which group measured the mass of the respective ion.